Think they are all overall very good casts, but heres my list:
1. Sean Connery, the 1st and best bond, ruthless, unforgiving, lethal and some crude humour
2 .Pierce Brosnan, very charming and charismatic bond, i really like hes performances, couple very entertaining films has well.
3 .Timothy Dalton, not very successful has bond but i really like hes dark and serious style, has well has one of my favorite films "Licence to Kill".
4 .Daniel Craig, good actor, 1st film was very good but the 2nd was painful to watch. Overall i like hes style although i think they focus too much on Bonds state of mind, when he is supposed to be a cold blooded ruthless and remorseless killer.
5 .Roger Moore, well he has some charm and charisma like Brosnan, but all of hes films are just horrible, with the womanizing and humorous bond getting out of control.
6. George Lazenby. Hes film is one of the best imo, but i just can't stand him.