Gotta say, Paragon VS Garrosh was great, probably because of how Jaz solo healed that. But yeah, any Paragon videos are usually very good. I enjoy Method one too, specially because they usually have their voice chat on and you can see how they can still have fun joking around early in the pull and still focus it down.
More old school, SK vs KJ was fantastic, the music fit perfectly with the boss dialogue